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Waste not, want not: CO2 (re)cycling into block polymers

Sumesh K. Raman, Robert Raja, Polly L. Arnold, Matthew G. Davidson, Charlotte K. Williams

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Abstract

A new way to combine two different polymerisation reactions, using a single catalyst, results in efficient block polymer synthesis. The selective polymerisation of mixtures of l-lactide-O-carboxyanhydride and cyclohexene oxide, using a di-zinc catalyst in a one-pot procedure, allows the preparation of poly(l-lactide-b-cyclohexene carbonate). The catalysis near quantitatively recycles the carbon dioxide released during polyester formation into the subsequent polycarbonate block, with an atom economy of up to of 91%.

Original languageEnglish
Pages (from-to)7315-7318
Number of pages4
JournalChemical Communications
Volume55
Issue number51
DOIs
Publication statusPublished - 2019

Bibliographical note

Publisher Copyright:
© The Royal Society of Chemistry 2019.

ASJC Scopus subject areas

  • Electronic, Optical and Magnetic Materials
  • Catalysis
  • Ceramics and Composites
  • General Chemistry
  • Surfaces, Coatings and Films
  • Metals and Alloys
  • Materials Chemistry

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