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Shining a light on Fe-catalyzed borrowing hydrogen alkylation

  • Salma A Elsherbeni
  • , Tahir Maqbool
  • , Md Abdul Bari
  • , Eman M. AlQahtani
  • , Louis C. Morrill
  • Cardiff University
  • Tanta University
  • Government College University Faisalabad

Research output: Contribution to journalReview articlepeer-review

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Abstract

The borrowing hydrogen (BH) approach enables commodity alcohols to be employed as alkylating agents, generating water as the sole by-product. Recently, Fe-based catalysts have been utilized in combination with visible light irradiation to enable alkylation processes at near room temperature, which improves sustainability metrics while presenting opportunities for further reaction development.
Original languageEnglish
Pages (from-to)168-170
Number of pages3
JournalTrends in Chemistry
Volume7
Issue number4
Early online date26 Feb 2025
DOIs
Publication statusPublished - 30 Apr 2025

Funding

The authors gratefully acknowledge the School of Chemistry at Cardiff University and the Department of Chemistry at the University of Bath for generous support. S.A.E. thanks the British Council and the Egyptian Cultural Affairs and Missions Sector for a PhD studentship through the Newton-Mosharafa Fund. T.M. thanks the Higher Education Commission of Pakistan Post-Doctoral Fellowship Programme (Phase III). E.M.A. thanks the Saudi Arabia Cultural Mission in the UK and the Department of Chemistry at King Khalid University, Saudi Arabia, for a PhD studentship. The authors declare no competing interests.

Funders
The British Council
Cardiff University
Egyptian Cultural Affairs and Missions Sector
Department of Chemistry at King Khalid University
Newton-Mosharafa Fund
University of Bath
Higher Education Commission

Keywords

  • alkylation
  • borrowing hydrogen
  • hydrogen autotransfer
  • iron catalysis
  • methylation
  • visible light

ASJC Scopus subject areas

  • General Chemistry

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