TY - JOUR
T1 - Relationship between vibrations and dynamical heterogeneity in a model glass former: Extended soft modes but local relaxation
AU - Ashton, D J
AU - Garrahan, J P
PY - 2009/11
Y1 - 2009/11
N2 - We study the relation between short-time vibrational modes and long-time relaxational dynamics in a kinetically constrained lattice gas with harmonic interactions between neighbouring particles. We find a correlation between the location of the low- (high-) frequency vibrational modes and regions of high (low) propensity for motion. This is similar to what was observed in continuous force systems, but our interpretation is different: in our case relaxation is due to localised excitations which propagate through the system; these localised excitations act as background disorder for the elastic network, giving rise to anomalous vibrational modes. Our results provide an example whereby a correlation between spatially extended low-frequency modes and high-propensity regions does not imply that relaxational dynamics originates in extended soft modes but rather belies their common origin. We consider other measures of elastic heterogeneity, such as non-affine displacement fields and mode localisation lengths, and discuss implications of our results to interpretations of dynamic heterogeneity more generally.
AB - We study the relation between short-time vibrational modes and long-time relaxational dynamics in a kinetically constrained lattice gas with harmonic interactions between neighbouring particles. We find a correlation between the location of the low- (high-) frequency vibrational modes and regions of high (low) propensity for motion. This is similar to what was observed in continuous force systems, but our interpretation is different: in our case relaxation is due to localised excitations which propagate through the system; these localised excitations act as background disorder for the elastic network, giving rise to anomalous vibrational modes. Our results provide an example whereby a correlation between spatially extended low-frequency modes and high-propensity regions does not imply that relaxational dynamics originates in extended soft modes but rather belies their common origin. We consider other measures of elastic heterogeneity, such as non-affine displacement fields and mode localisation lengths, and discuss implications of our results to interpretations of dynamic heterogeneity more generally.
UR - http://www.scopus.com/inward/record.url?scp=72549112251&partnerID=8YFLogxK
UR - http://dx.doi.org/10.1140/epje/i2009-10531-6
U2 - 10.1140/epje/i2009-10531-6
DO - 10.1140/epje/i2009-10531-6
M3 - Article
SN - 0253-2786
VL - 30
SP - 303
EP - 307
JO - The European Physical Journal E - Soft Matter
JF - The European Physical Journal E - Soft Matter
IS - 3
ER -