Near infrared ultrafast pump-probe spectroscopy with ZrF4-BaF2-LaF3-AlF3-NaF fiber supercontinuum

Stefan Fischbach, Andrey V. Gorbach, Daniele Di Nuzzo, Enrico Da Como

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Abstract

We report on the performance of a setup designed for femtosecond pump-probe spectroscopy in the near infrared (NIR) spectral region. We generate a supercontinuum (SC) probe by coupling 140 fs light pulses at 1550 nm into a ZrF4-BaF2-LaF3-AlF3-NaF (ZBLAN) fiber. The combined high nonlinearity and transparency of the ZBLAN fluoride glass allows us to obtain a SC probe from 1 to 2.6 μm. The NIR pulses are used to demonstrate a proof of principle experiment probing the relaxation of photo induced excitations in a conjugated polymer:fullerene blend film. The results show the possibility to perform fibre based NIR SC femtosecond spectroscopy at >100 KHz repetition rate and using lasers with pulse energy just above 300 nJ.
Original languageEnglish
Article number021103
Pages (from-to)1 - 4
Number of pages4
JournalApplied Physics Letters
Volume107
Issue number2
Early online date14 Jul 2015
DOIs
Publication statusPublished - 14 Jul 2015

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pumps
fibers
probes
pulses
spectroscopy
fullerenes
fluorides
repetition
nonlinearity
glass
polymers
excitation
lasers
energy

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Near infrared ultrafast pump-probe spectroscopy with ZrF4-BaF2-LaF3-AlF3-NaF fiber supercontinuum. / Fischbach, Stefan; Gorbach, Andrey V.; Di Nuzzo, Daniele; Da Como, Enrico.

In: Applied Physics Letters, Vol. 107, No. 2, 021103, 14.07.2015, p. 1 - 4.

Research output: Contribution to journalArticle

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