An overview of CO2 capture technologies

Niall MacDowell, Nick Florin, Antoine Buchard, Jason Hallett, Amparo Galindo, George Jackson, Claire S. Adjiman, Charlotte K. Williams, Nilay Shah, Paul Fennell

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Abstract

In this paper, three of the leading options for large scale CO2 capture are reviewed from a technical perspective. We consider solvent-based chemisorption techniques, carbonate looping technology, and the so-called oxyfuel process. For each technology option, we give an overview of the technology, listing advantages and disadvantages. Subsequently, a discussion of the level of technological maturity is presented, and we conclude by identifying current gaps in knowledge and suggest areas with significant scope for future work. We then discuss the suitability of using ionic liquids as novel, environmentally benign solvents with which to capture CO2. In addition, we consider alternatives to simply sequestering CO2-we present a discussion on the possibility of recycling captured CO2 and exploiting it as a C1 building block for the sustainable manufacture of polymers, fine chemicals, and liquid fuels. Finally, we present a discussion of relevant systems engineering methodologies in carbon capture system design.
Original languageEnglish
Pages (from-to)1645-1669
Number of pages25
JournalEnergy & Environmental Science
Volume3
Issue number11
Early online date31 Aug 2010
DOIs
Publication statusPublished - 2010

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Carbon Monoxide
Ionic Liquids
Carbon capture
Carbonates
Liquid fuels
Chemisorption
Systems engineering
Ionic liquids
Recycling
Polymers
recycling
polymer
Systems analysis
carbonate
engineering
liquid
methodology
carbon

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MacDowell, N., Florin, N., Buchard, A., Hallett, J., Galindo, A., Jackson, G., ... Fennell, P. (2010). An overview of CO2 capture technologies. Energy & Environmental Science, 3(11), 1645-1669. https://doi.org/10.1039/C004106H

An overview of CO2 capture technologies. / MacDowell, Niall; Florin, Nick; Buchard, Antoine; Hallett, Jason; Galindo, Amparo; Jackson, George; Adjiman, Claire S.; Williams, Charlotte K.; Shah, Nilay; Fennell, Paul.

In: Energy & Environmental Science, Vol. 3, No. 11, 2010, p. 1645-1669.

Research output: Contribution to journalArticle

MacDowell, N, Florin, N, Buchard, A, Hallett, J, Galindo, A, Jackson, G, Adjiman, CS, Williams, CK, Shah, N & Fennell, P 2010, 'An overview of CO2 capture technologies', Energy & Environmental Science, vol. 3, no. 11, pp. 1645-1669. https://doi.org/10.1039/C004106H
MacDowell N, Florin N, Buchard A, Hallett J, Galindo A, Jackson G et al. An overview of CO2 capture technologies. Energy & Environmental Science. 2010;3(11):1645-1669. https://doi.org/10.1039/C004106H
MacDowell, Niall ; Florin, Nick ; Buchard, Antoine ; Hallett, Jason ; Galindo, Amparo ; Jackson, George ; Adjiman, Claire S. ; Williams, Charlotte K. ; Shah, Nilay ; Fennell, Paul. / An overview of CO2 capture technologies. In: Energy & Environmental Science. 2010 ; Vol. 3, No. 11. pp. 1645-1669.
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