An efficient low-temperature route to nitrogen-doping and activation of mesoporous carbons for CO2 capture

Kuan Huang; Song Hai Chai; Richard T. Mayes; Gabriel M. Veith; Katie L. Browning; Miles A. Sakwa-Novak; Matthew E. Potter; Christopher W. Jones; You Ting Wu; Sheng Dai

doi:10.1039/c5cc05619e

An efficient low-temperature route to nitrogen-doping and activation of mesoporous carbons for CO₂ capture

Kuan Huang, Song Hai Chai, Richard T. Mayes, Gabriel M. Veith, Katie L. Browning, Miles A. Sakwa-Novak, Matthew E. Potter, Christopher W. Jones, You Ting Wu, Sheng Dai

Research output: Contribution to journal › Article › peer-review

56 Citations (SciVal)

Abstract

An innovative strategy for post-synthesis nitrogen-doping of mesoporous carbons (MCs) with high yields (>90%) at low temperatures (230-380 °C) by using a strong base, sodium amide (NaNH₂), was developed. The as-prepared N-doped MCs exhibit a significantly enhanced CO₂ adsorption performance in terms of capacity and selectivity when compared to their parent MCs.

Original language	English
Pages (from-to)	17261-17264
Number of pages	4
Journal	Chemical Communications
Volume	51
Issue number	97
Early online date	29 Sept 2015
DOIs	https://doi.org/10.1039/c5cc05619e
Publication status	Published - 18 Dec 2015

Bibliographical note

Publisher Copyright:
© The Royal Society of Chemistry.

Funding

Funders	Funder number
China Scholarship Council
National Natural Science Foundation of China	21376115
Parliamentary Office of Science and Technology
US Department of Energy	DE-SC0012577

ASJC Scopus subject areas

Electronic, Optical and Magnetic Materials
Catalysis
Ceramics and Composites
General Chemistry
Surfaces, Coatings and Films
Metals and Alloys
Materials Chemistry

Access to Document

10.1039/c5cc05619eLicence: Unspecified

Cite this

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abstract = "An innovative strategy for post-synthesis nitrogen-doping of mesoporous carbons (MCs) with high yields (>90\%) at low temperatures (230-380 °C) by using a strong base, sodium amide (NaNH2), was developed. The as-prepared N-doped MCs exhibit a significantly enhanced CO2 adsorption performance in terms of capacity and selectivity when compared to their parent MCs.",

author = "Kuan Huang and Chai, \{Song Hai\} and Mayes, \{Richard T.\} and Veith, \{Gabriel M.\} and Browning, \{Katie L.\} and Sakwa-Novak, \{Miles A.\} and Potter, \{Matthew E.\} and Jones, \{Christopher W.\} and Wu, \{You Ting\} and Sheng Dai",

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AU - Huang, Kuan

AU - Chai, Song Hai

AU - Mayes, Richard T.

AU - Veith, Gabriel M.

AU - Browning, Katie L.

AU - Sakwa-Novak, Miles A.

AU - Potter, Matthew E.

AU - Jones, Christopher W.

AU - Wu, You Ting

AU - Dai, Sheng

PY - 2015/12/18

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