A comparison between monolithic and wire gauze structured catalytic reactors for CH4 and CO removal from biogas-fuelled engine exhaust

P.J. Jodłowski; R. Goła̧b; J. Kryca; A. Kołodziej; M. Iwaniszyn; S.T. Kolaczkowski; J. Łojewska

doi:10.1007/s11244-013-9985-5

A comparison between monolithic and wire gauze structured catalytic reactors for CH₄ and CO removal from biogas-fuelled engine exhaust

P.J. Jodłowski, R. Goła̧b, J. Kryca, A. Kołodziej, M. Iwaniszyn, S.T. Kolaczkowski, J. Łojewska

Research output: Contribution to journal › Article › peer-review

12 Citations (SciVal)

163 Downloads (Pure)

Abstract

The application of the wire gauzes as the catalytic supports can provide a number of advantages in biogas exhaust abatement. In this paper, a model of wire gauze structured reactor for biogas exhaust removal is proposed and model based calculations are performed to compare the wire gauze catalytic reactor with the classic monolith. The modelling bases on kinetic data experimentally obtained in a small-scale tubular reactor for cobalt and palladium (as reference) oxide catalysts doped with promoters (Ce, Pd). The heat and mass transfer characteristics of the wire gauze reactor are taken from the former studies by the authors. The simulations show that for assumed reactor parameters, a combination of the promoted cobalt oxide catalyst and the wire gauze support can give high conversion of methane and carbon monoxide.

Original language	English
Pages (from-to)	390-396
Number of pages	7
Journal	Topics in Catalysis
Volume	56
Issue number	1-8
DOIs	https://doi.org/10.1007/s11244-013-9985-5
Publication status	Published - May 2013

Access to Document

10.1007/s11244-013-9985-5

10.1007_s11244-013-9985-5
This article is distributed under the terms of the Creative Commons Attribution License which permits any use, dis- tribution, and reproduction in any medium, provided the original author(s) and the source are credited
Final published version, 339 KBLicence: CC BY

Cite this

@article{8836d5ee1abf4c6aa68c8250a4e9bec9,

title = "A comparison between monolithic and wire gauze structured catalytic reactors for CH4 and CO removal from biogas-fuelled engine exhaust",

abstract = "The application of the wire gauzes as the catalytic supports can provide a number of advantages in biogas exhaust abatement. In this paper, a model of wire gauze structured reactor for biogas exhaust removal is proposed and model based calculations are performed to compare the wire gauze catalytic reactor with the classic monolith. The modelling bases on kinetic data experimentally obtained in a small-scale tubular reactor for cobalt and palladium (as reference) oxide catalysts doped with promoters (Ce, Pd). The heat and mass transfer characteristics of the wire gauze reactor are taken from the former studies by the authors. The simulations show that for assumed reactor parameters, a combination of the promoted cobalt oxide catalyst and the wire gauze support can give high conversion of methane and carbon monoxide. ",

author = "P.J. Jod{\l}owski and R. Go{\l}{\c a}b and J. Kryca and A. Ko{\l}odziej and M. Iwaniszyn and S.T. Kolaczkowski and J. {\L}ojewska",

year = "2013",

month = may,

doi = "10.1007/s11244-013-9985-5",

language = "English",

volume = "56",

pages = "390--396",

journal = "Topics in Catalysis",

issn = "1022-5528",

publisher = "Springer",

number = "1-8",

}

TY - JOUR

T1 - A comparison between monolithic and wire gauze structured catalytic reactors for CH4 and CO removal from biogas-fuelled engine exhaust

AU - Jodłowski, P.J.

AU - Goła̧b, R.

AU - Kryca, J.

AU - Kołodziej, A.

AU - Iwaniszyn, M.

AU - Kolaczkowski, S.T.

AU - Łojewska, J.

PY - 2013/5

Y1 - 2013/5

N2 - The application of the wire gauzes as the catalytic supports can provide a number of advantages in biogas exhaust abatement. In this paper, a model of wire gauze structured reactor for biogas exhaust removal is proposed and model based calculations are performed to compare the wire gauze catalytic reactor with the classic monolith. The modelling bases on kinetic data experimentally obtained in a small-scale tubular reactor for cobalt and palladium (as reference) oxide catalysts doped with promoters (Ce, Pd). The heat and mass transfer characteristics of the wire gauze reactor are taken from the former studies by the authors. The simulations show that for assumed reactor parameters, a combination of the promoted cobalt oxide catalyst and the wire gauze support can give high conversion of methane and carbon monoxide.

AB - The application of the wire gauzes as the catalytic supports can provide a number of advantages in biogas exhaust abatement. In this paper, a model of wire gauze structured reactor for biogas exhaust removal is proposed and model based calculations are performed to compare the wire gauze catalytic reactor with the classic monolith. The modelling bases on kinetic data experimentally obtained in a small-scale tubular reactor for cobalt and palladium (as reference) oxide catalysts doped with promoters (Ce, Pd). The heat and mass transfer characteristics of the wire gauze reactor are taken from the former studies by the authors. The simulations show that for assumed reactor parameters, a combination of the promoted cobalt oxide catalyst and the wire gauze support can give high conversion of methane and carbon monoxide.

UR - http://www.scopus.com/inward/record.url?scp=84877939387&partnerID=8YFLogxK

UR - http://dx.doi.org/10.1007/s11244-013-9985-5

UR - http://link.springer.com/article/10.1007%2Fs11244-013-9985-5

U2 - 10.1007/s11244-013-9985-5

DO - 10.1007/s11244-013-9985-5

M3 - Article

AN - SCOPUS:84877939387

SN - 1022-5528

VL - 56

SP - 390

EP - 396

JO - Topics in Catalysis

JF - Topics in Catalysis

IS - 1-8

ER -

A comparison between monolithic and wire gauze structured catalytic reactors for CH₄ and CO removal from biogas-fuelled engine exhaust

Abstract

Access to Document

Other files and links

Fingerprint

Cite this